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8.611 Aktuelle Fachpublikationen in Inorganic Chemistry


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Transition-Metal-Complex Cationic Dyes Photosensitive to Two Types of 2D Layered Silver Bromides with Visible-Light-Driven Photocatalytic Properties

23.11.2016 | Cheng-Yang Yue; Xiao-Wu Lei; Yong-Fang Han; Xin-Xiu Lu; Ya-Wei Tian; Jing Xu; Xiao-Fan Liu; Xin Xu, Inorganic Chemistry, 2016

With mixed transition-metal (TM) complex, alkali-metal cations, or halogen anions as structure-directing agents, two types of two-dimensional (2D) layered inorganic–organic hybrid silver bromides were prepared and structurally characterized as K[TM(2,2-bipy)3]2Ag6Br11 (TM = Ni (1), Co (2), Zn ...


Significantly Dense Two-Dimensional Hydrogen-Bond Network in a Layered Zirconium Phosphate Leading to High Proton Conductivities in Both Water-Assisted Low-Temperature and Anhydrous Intermediate-Temperature Regions

23.11.2016 | Daxiang Gui; Tao Zheng; Jian Xie; Yawen Cai; Yaxing Wang; Lanhua Chen; Juan Diwu; Zhifang Chai; Shuao Wang, Inorganic Chemistry, 2016

Inorganic Chemistry DOI: 10.1021/acs.inorgchem.6b02308


“Straining” to Separate the Rare Earths: How the Lanthanide Contraction Impacts Chelation by Diglycolamide Ligands

23.11.2016 | Ross J. Ellis; Derek M. Brigham; Laetitia Delmau; Alexander S. Ivanov; Neil J. Williams; Minh Nguyen Vo; Benjamin Re ..., Inorganic Chemistry, 2016

The subtle energetic differences underpinning adjacent lanthanide discrimination are explored with diglycolamide ligands. Our approach converges liquid–liquid extraction experiments with solution-phase X-ray absorption spectroscopy (XAS) and density functional theory (DFT) simulations, spanning ...


Selective Carbon Dioxide Adsorption by Two Robust Microporous Coordination Polymers

23.11.2016 | Litao An; Hao Wang; Feng Xu; Xin-Long Wang; Fangming Wang; Jing Li, Inorganic Chemistry, 2016

In the present work we report the design, synthesis, crystal structure determination, and adsorption properties of two new cadmium-based porous coordination polymers, [Cd(pda)0.5(spiro-4-py)0.5(HCOO)]·2H2O·DMF (compound 1, pda = p-phenylenediacetate, spiro-4-py = ...


Rare Neutral Diphosphine Complexes of Scandium(III) and Yttrium(III) Halides

23.11.2016 | Marina Carravetta; Maria Concistre; William Levason; Gillian Reid; Wenjian Zhang, Inorganic Chemistry, 2016

Reaction of Me2PCH2CH2PMe2 or o-C6H4(PMe2)2 (L–L) with a suspension of ScI3 or YI3 in MeCN solution under rigorously anhydrous and oxygen-free conditions produced the highly unusual complexes [ScI3(L–L)2], [YI3(Me2PCH2CH2PMe2)2], and [YI3{o-C6H4(PMe2)2}2MeCN]. X-ray crystal structures reveal that ...


Manganese Tricarbonyl Complexes with Asymmetric 2-Iminopyridine Ligands: Toward Decoupling Steric and Electronic Factors in Electrocatalytic CO2 Reduction

23.11.2016 | Steven J. P. Spall; Theo Keane; Joanne Tory; Dean C. Cocker; Harry Adams; Hannah Fowler; Anthony J. H. M. Meijer; Fr ..., Inorganic Chemistry, 2016

Manganese tricarbonyl bromide complexes incorporating IP (2-(phenylimino)pyridine) derivatives, [MnBr(CO)3(IP)], are demonstrated as a new group of catalysts for CO2 reduction, which represent the first example of utilization of (phenylimino)pyridine ligands on manganese centers for this purpose. ...


Instability of the Ionic Conductor Li6BaLa2B2O12 (B = Nb, Ta): Barium Exsolution from the Garnet Network Leading to CO2 Capture

23.11.2016 | Cyrille Galven; Gwenaël Corbel; Françoise Le Berre; Marie-Pierre Crosnier-Lopez, Inorganic Chemistry, 2016

The instability of the two garnets Li6BaLa2B2O12 (B = Nb, Ta) has been studied on samples prepared in powder form by solid-state reaction. For this study, we coupled different techniques: powder X-ray diffraction, IR spectrometry, thermal analysis, transmission electron microscopy, and complex ...


Effect of Internal Pressure and Temperature on Phase Transitions in Perovskite Oxides: The Case of the Solid Oxide Fuel Cell Cathode Materials of the La2–xSrxCoTiO6 Series

23.11.2016 | Alejandro Gómez-Pérez; Markus Hoelzel; Álvaro Muñoz-Noval; Flaviano García-Alvarado; Ulises Amador, Inorganic Chemistry, 2016

The symmetry of the room-temperature (RT) structure of title compounds La2–xSrxCoTiO6−δ changes with x, from P21/n (0 ≤ x ≤ 0.2) to Pnma (0.3 ≤ x ≤ 0.5) and to R3̅c (0.6 ≤ x ≤ 1). For x = 1 the three pseudocubic cell parameters become very close suggesting a transition to a cubic structure for ...


Computational Gas-Phase Formation Enthalpy and Electron Affinity for Platinum Hexafluoride: Is Gaseous PtF6 Diamagnetic because of a Relativistic Effect?

23.11.2016 | Robson Fernandes De Farias, Inorganic Chemistry, 2016

In the present work, a computational thermochemistry study (semiempirical, PM6 method) for platinum hexafluoride (PtF6) is performed. The gas-phase formation enthalpy (ΔfH°) and electron affinity are calculated and the results compared with the experimental data. A calculated ΔfH°(g) value of ...


Transformation of One-Dimensional Achiral Structure to Three-Dimensional Chiral Structure: Mechanistic Study and Catalytic Activities of Chiral Structure

23.11.2016 | Purna Chandra Rao; Sonu Pratap Chaudhary; Denis Kuznetsov; Sukhendu Mandal, Inorganic Chemistry, 2016

We have isolated two copper-based coordination polymers through solvent diffusion and solvothermal methods using copper salt, furan dicarboxylic acid (FDC), 4,4′-bipyridine (bpy) in MeOH/ethylene glycol, and water solvents. Compound 1 is adopting P21/c space group and adopts a one-dimensional ...


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