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6.171 Aktuelle Fachpublikationen in Inorganic Chemistry

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Synthesis of Phase-Pure U2N3 Microspheres and Its Decomposition into UN

12.12.2014 | Chinthaka M. Silva; Rodney D. Hunt; Lance L. Snead; Kurt A. Terrani, Inorganic Chemistry, 2014

Uranium mononitride (UN) is important as a nuclear fuel. Fabrication of UN in its microspherical form also has its own merits since the advent of the concept of accident-tolerant fuel, where UN is being considered as a potential fuel in the form of TRISO particles. However, not many processes ...

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A Diferrous Dithiolate as a Model of the Elusive Hoxinact State of the [FeFe] Hydrogenases: An Electrochemical and Theoretical Dissection of Its Redox Chemistry

12.12.2014 | Dounia Chouffai; Jean-François Capon; Luca De Gioia; François Y. Pétillon; Philippe Schollhammer; Jean Talarmin; Giu ..., Inorganic Chemistry, 2014

The reduction of the Fe(II)Fe(II) complex [Fe2(CO)2{P(OMe)3}2(κ2-IMe-CH2-IMe)(μ-CO)(μ-pdt)]2+ (2P2+; pdt = S(CH2)3S), which is a synthetic model of the H cluster of the [FeFe] hydrogenases in its inactive state, has been investigated electrochemically and theoretically (by density functional ...

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Differences in the Binding of Copper(I) to α- and β-Synuclein

12.12.2014 | Riccardo De Ricco; Daniela Valensin; Simone Dell’Acqua; Luigi Casella; Elena Gaggelli; Gianni Valensin; Luigi Bubacc ..., Inorganic Chemistry, 2014

Parkinson’s disease (PD) is a neurodegenerative disorder characterized by the presence of abnormal α-synuclein (αS) deposits in the brain. Alterations in homeostasis and metal-induced oxidative stress may play a crucial role in the progression of αS amyloid assembly and pathogenesis of PD. ...

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Electronic Effects of Ligand Substitution on Spin Crossover in a Series of Diiminoquinonoid-Bridged FeII2 Complexes

12.12.2014 | Jesse G. Park; Ie-Rang Jeon; T. David Harris, Inorganic Chemistry, 2014

A series of four isostructural FeII2 complexes, [(TPyA)2Fe2(XL)]2+ (TPyA = tris(2-pyridylmethyl)amine; XL2– = doubly deprotonated form of 3,6-disubstituted-2,5-dianilino-1,4-benzoquinone; X = H, Br, Cl, and F), were synthesized to enable a systematic study of electronic effects on spin crossover ...

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2-(Phenylazo)pyridineplatinum(II) Catecholates Showing Photocytotoxicity, Nuclear Uptake, and Glutathione-Triggered Ligand Release

12.12.2014 | Koushambi Mitra; Shilpa Patil; Paturu Kondaiah; Akhil R. Chakravarty, Inorganic Chemistry, 2014

Platinum(II) complexes [Pt(pap)(an-cat)] (1) and [Pt(pap)(py-cat)] (2) with 2-(phenylazo)pyridine (pap), 4-[2-[(anthracen-9-ylmethylene)amino]ethyl]benzene-1,2-diol (H2an-cat), and 4-[2-[(pyren-1-ylmethylene)amino]ethyl]benzene-1,2-diol (H2py-cat) were prepared, and their photoinduced ...

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A Series of MIICuII3 Stars (M = Mn, Ni, Cu, Zn) Exhibiting Unusual Magnetic Properties

12.12.2014 | Suraj Mondal; Shuvankar Mandal; Luca Carrella; Arpita Jana; Michel Fleck; Andreas Köhn; Eva Rentschler; Sasankasekha ..., Inorganic Chemistry, 2014

The work in this report describes the syntheses, electrospray ionization mass spectromtery, structures, and experimental and density functional theoretical (DFT) magnetic properties of four tetrametallic stars of composition [MII(CuIIL)3](ClO4)2 (1, M = Mn; 2, M = Ni; 3, M = Cu; 4, M = Zn) ...

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Field-Induced Slow Relaxation in a Monometallic Manganese(III) Single-Molecule Magnet

12.12.2014 | Gavin A. Craig; Jonathan J. Marbey; Stephen Hill; Olivier Roubeau; Simon Parsons; Mark Murrie, Inorganic Chemistry, 2014

Inorganic Chemistry DOI: 10.1021/ic5024136

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Potential Switchable Circularly Polarized Luminescence from Chiral Cyclometalated Platinum(II) Complexes

11.12.2014 | Xiao-Peng Zhang; Victoria Y. Chang; Jian Liu; Xiao-Liang Yang; Wei Huang; Yizhi Li; Cheng-Hui Li; Gilles Muller; Xia ..., Inorganic Chemistry, 2014

A series of chiral cyclometalated platinum(II) complexes, [Pt((−)-L1)(Dmpi)]Cl ((−)-1), [Pt((+)-L1)(Dmpi)]Cl ((+)-1), [Pt((−)-L2)(Dmpi)]Cl ((−)-2), [Pt((+)-L2)(Dmpi)]Cl ((+)-2), [Pt3((−)-L2)2(Dmpi)4](ClO4)4 ((−)-3), and [Pt3((+)-L2)2(Dmpi)4](ClO4)4 ((+)-3) [(−)-L1 = ...

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Host-Sensitized Luminescence Properties in CaNb2O6:Ln3+ (Ln3+ = Eu3+/Tb3+/Dy3+/Sm3+) Phosphors with Abundant Colors

11.12.2014 | Kai Li; Xiaoming Liu; Yang Zhang; Xuejiao Li; Hongzhou Lian; Jun Lin, Inorganic Chemistry, 2014

A series of Ln3+ (Ln3+ = Eu3+/Tb3+/Dy3+/Sm3+) ion doped CaNb2O6 (CNO) phosphors have been prepared via the conventional high-temperature solid-state reaction route. The X-ray diffraction (XRD) and structure refinement, diffuse reflection, photoluminescence (PL), and fluorescent decay curves were ...

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Near-IR Luminescence and Field-Induced Single Molecule Magnet of Four Salen-type Ytterbium Complexes

11.12.2014 | Tian-Qi Liu; Peng-Fei Yan; Fang Luan; Yu-Xin Li; Jing-Wen Sun; Chuan Chen; Fan Yang; Han Chen; Xiao-Yan Zou; Guang-M ..., Inorganic Chemistry, 2014

A series of rigid hexadentate salen-type (H2L) ytterbium complexes, namely, [Yb2L3(CH3OH)]·3CH3CN (1), [Yb2LL′L″(CH3OH)(H2O)2](ClO4)2·CH3OH·H2O (2), [Yb2L(OAc)4(CH3OH)2]·2CH3OH (3), and {[Yb2L(OAc)4]·3H2O}n (4) (H2L = N,N′-bis(2-oxy-3-methoxybenzylidene)-1,2-phenylenediamine, HL′ = ...

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