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Charge effects regulate reversible CO2 reduction catalysis

Modular but geometrically constrained ligands were used to investigate the impact of key ligand design parameters (charge and bite angle) on CO2 hydrogenation and formic acid dehydrogenation activity. These studies yielded an optimized catalyst that achieved over 118 000 turnovers in CO2 hydrogenation, 247 000 turn

Autoren:   Jacob B. Geri; Joanna L. Ciatti; Nathaniel K. Szymczak
Journal:   Chemical Communication
DOI:   10.1039/C8CC04370A
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