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Spin-coating-assisted fabrication of ultrathin physical hydrogel films with high toughness and fast response

03.07.2018 | Si Yu Zheng; Ye Tian; Xin Ning Zhang; Miao Du; Yihu Song; Zi Liang Wu; Qiang Zheng, Soft Matter, 2018

Hydrogel films have promising applications in medical dressings, flexible electronics, etc. However, it is challenging to fabricate ultrathin hydrogel films with high toughness and controllable thickness. Here, we report a facile approach to prepare tough physical hydrogel films by spin-coating ...

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Geometric distortions in nickel (oxy)hydroxide electrocatalysts by redox inactive iron ions

03.07.2018 | Rodney D. L. Smith; Chiara Pasquini; Stefan Loos; Petko Chernev; Katharina Klingan; Paul Kubella; Mohammad Reza Moha ..., Energy & Environmental Science, 2018

The dramatic change in electrochemical behavior of nickel (oxy)hydroxide films upon incorporation of Fe ions provides an opportunity to establish effective electrocatalyst design principles. We characterize a photochemically deposited series of Fe–Ni (oxy)hydroxides by X-ray absorption ...

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Correction: Neutron diffraction studies on the thermal expansion and anomalous mechanics in the perovskite-type [C(ND2)3]Me2+(DCOO)3 [Me = Cu, Mn, Co]

03.07.2018 | M. Viswanathan, Physical Chemistry Chemical Physics, 2018

Correction for ‘Neutron diffraction studies on the thermal expansion and anomalous mechanics in the perovskite-type [C(ND2)3]Me2+(DCOO)3 [Me = Cu, Mn, Co]’ by M. Viswanathan et al., Phys. Chem. Chem. Phys., 2018, DOI: 10.1039/c8cp01245h.

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Doping stability of nonphotorefractive ions in stoichiometric and congruent LiNbO3

03.07.2018 | Lili Li; Yanlu Li; Xian Zhao, Physical Chemistry Chemical Physics, 2018

The doping stability of various nonphotorefractive ions including Mg, Zn, In, Sc, Sn, Hf, and Zr in stoichiometric, congruent, and Fe-doped LiNbO3 has been investigated by hybrid density functional theory. It is found to be energetically prefer for all the dopants to incorporate into Li sites of ...

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Creating Capsules with Cubanes

03.07.2018 | Sotaro Kusumoto; Fumiya Kobayashi; Ryo Ohtani; Yingjie Zhang; J. M. Harrowfield; Yang Kim; Shinya Hayami; Masaaki N ..., Dalton Transactions, 2018

A sextuply linked capsule incorporating two Ni(II) cubane units is formed when Ni(II) salts are reacted with N-aminoalkyl salicylamidato ligands in a 4:3 ratio in methanol. With a short (propyl) alkyl substituent, additional chloride counter ions are included in the cavity by occupation of one ...

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Novel magnetite nanorods decorated Si-Schiff base complex for efficient immobilization of U(VI) and Pb(II) from water solutions

03.07.2018 | Xiangke Wang; Ayub Khan; JINLU XING; Ahmed Mourtada Elseman; Pengcheng Gu; Kashif Gul; Yuejie Ai; Riffat Jehan; Ahme ..., Dalton Transactions, 2018

A novel silicon Schiff base complex (Si-SBC) and magnetite nanorods decorated Si-SBC (M/SiO2-Si-SBC) were synthesized and well characterized in detail. The synthesized materials were applied for the removal of U(VI) and Pb(II) from water solutions under various experimental conditions. The ...

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In Silico Study of Bombyx Mori Fibroin Enhancement by Graphene in Acidic Environment

03.07.2018 | Duy Phuoc Tran; Vi Toan Lam; Tan Lien Tran; Thuy Nhu Son Nguyen; Hanh Thi Thu Tran, Physical Chemistry Chemical Physics, 2018

Bombyx Mori Fibroin has been widely used long time ago and becoming popular materials. Here, we carry out the Molecular Dynamics simulation based docking simulation of small fragment of graphene in order to seek for the best binding position on the N-termini domain of Bombyx Mori fibroin. We ...

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Design Concepts in Absorbance Optical Systems for Analytical Ultracentrifugation

03.07.2018 | Joseph Pearson; Marcel Hofstetter; Thomas Dekorsy; Michael Totzeck; Helmut Coelfen, Analyst, 2018

Analytical ultracentrifugation is a powerful technique for analyzing particles in solution, and has proved valuable for a wide range of applications in chemistry, biochemistry and material sciences for many years. The field is presently seeing a resurgence of instrument development from ...

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Molecular dynamics simulation of the electrical conductive network formation of polymer nanocomposites with polymer-grafted nanorod

03.07.2018 | Fanzhu Li; Xiaohui Duan; Huan Zhang; Bin Li; Jun Liu; Yangyang Gao; Liqun Zhang, Physical Chemistry Chemical Physics, 2018

Grafting chains on the surface of filler is an effective strategy to tune and control the filler conductive network, which can be utilized to fabricate polymer nanocomposites (PNCs) with high electrical conductivity. In this work, by employing the coarse-grained molecular dynamics simulation, we ...

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Synthesis of cationic molybdenum-cobalt heterometallic clusters protected against hydrolysis by macrocyclic triazacyclononane complexes

03.07.2018 | Sugiarto .; Tomoko Tagami; Keisuke Kawamoto; Yoshihito Hayashi, Dalton Transactions, 2018

Four kinds of cobalt-polyoxomolybdenum clusters were synthesized by a combination of polyoxomolybdates and a Co-tacn (tacn = 1,4,7-triazacyclononane) complex. The heterometallic polynuclear clusters were obtained by the reaction of Na2MoO4 and [Co(tacn)(H2O)3](CF3SO3)3∙H2O in aqueous solution. ...

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